Hayley Atwell Agent Peggy Carter Actor James D'Arcy Edwin Jarvis Actor Chad Michael Murray Agent Jack Thompson Actor Enver Gjokaj Agent Daniel Sousa Actor Shea Whigham Chief Roger Dooley Actor Lyndsy Fonseca Guest Star James Herbert Guest Star Kyle Bornheimer Guest Star James Frain Guest Star Erin Torpey Guest Star Walker Roach Guest Star Greg Bryan Guest Star Ray Wise Guest Star Meagen Fay Guest Star James Urbaniak Guest Star Devin Ratray Guest Star Ralph Garman Guest Star Don Luce Guest Star Jeff Locker Guest Star Atticus Todd Guest Star Tara Butters Executive Producer Michele Fazekas Executive Producer Christopher Markus Executive Producer Stephen McFeely Executive Producer Chris Dingess Executive Producer Kevin Feige Executive Producer Louis D'Esposito Executive Producer Alan Fine Executive Producer Joe Quesada Executive Producer Stan Lee Executive Producer Jeph Loeb Executive Producer Eric Pearson Writer Joe Russo Director