Robert Vaughn Napolean Solo Actor David McCallum Illya Kuryakin Actor Leo G. Carroll Mr. Alexander Waverly Actor Danielle De Metz Guest Star Herbert Lom Guest Star Jeannine Riley Guest Star Eduardo Ciannelli Guest Star Curd Jürgens Guest Star Philip Ahn Guest Star Telly Savalas Guest Star Jack La Rue Guest Star Peggy Ann Taylor Guest Star Richard Angarola Guest Star Fritz Feld Guest Star Letícia Román Guest Star Dave Armstrong Guest Star Sharyn Hillyer Guest Star Stuart Nisbet Guest Star Dick Crockett Guest Star Slapsy Maxie Rosenbloom Guest Star Norman Felton Executive Producer David Victor Producer Boris Ingster Producer, Writer Irving Pearlberg Producer Stanford Sherman Writer Robert Hill Writer John Brahm Director Berne Giler Writer Harlan Ellison Writer Sherman Marks Director Joseph Sargent Director E. Darrell Hallenbeck Director Barry Shear Director Norman Hudis Writer Joseph Cavella Writer Peter Allan Fields Writer Don Richman Writer George Waggner Director Stanley Ralph Ross Writer