Jon Bokenkamp Creator James Spader Raymond "Red" Reddington Actor, Executive Producer Diego Klattenhoff Donald Ressler Actor Amir Arison Aram Mojtabai Actor Hisham Tawfiq Dembe Zuma Actor Harry Lennix Harold Cooper Actor Laura Sohn Alina Park Actor Jonathan Holtzman Chuck Guest Star Lukas Hassel Elias Vandyke Guest Star Fisher Stevens Marvin Gerard Guest Star Ross Partridge Reggie Cole Guest Star Karina Arroyave Mierce Xiu Guest Star Diany Rodriguez Weecha Xiu Guest Star Teagle F. Bougere Tyson Lacroix Guest Star Ivan Moore Alvarez Guest Star Taylor Green Esther Guest Star Pawel Szajda Henrick Fisker Guest Star Kaye Tuckerman Hildebrand Guest Star Melissa Hunter McCann Polly Guest Star Mario Peguero Santiago Guest Star Tyler French Commando Guest Star Opal Besson Female Crime Boss Guest Star John Squires Male Crime Boss Guest Star Katina Forté Operations Manager Guest Star Andrew Haserlat Tech Expert Guest Star John Eisendrath Executive Producer John Davis Executive Producer John Fox Executive Producer Lukas Reiter Executive Producer J.R. Orci Executive Producer Laura Benson Executive Producer Christine Moore Director Daniel Cerone Writer