Robert Vaughn Napolean Solo Actor David McCallum Illya Kuryakin Actor Leo G. Carroll Mr. Alexander Waverly Actor Jill Ireland Guest Star Glenn Corbett Guest Star Anne Francis Guest Star Danica D'Hondt Guest Star May Heatherly Guest Star Ted Roter Guest Star Leigh Chapman Guest Star John Van Dreelen Guest Star Charles Giorgi Guest Star Ben Wright Guest Star Dinny Powell Guest Star Erik Holland Guest Star Kathy Kersh Guest Star Nancy Kovack Guest Star Miguel Ángel Landa Guest Star Hedley Mattingly Guest Star George Sawaya Guest Star Norman Felton Executive Producer Theodore J. Flicker Director Sam Rolfe Producer Alvin Ganzer Director Richard Donner Director Peter Allan Fields Writer Marc Daniels Director Joseph Sargent Director Albert Aley Writer Ellis Marcus Writer Anthony Spinner Writer Ron Winston Director Alan Caillou Writer Dick Nelson Writer John Peyser Director Dean Hargrove Writer Aben Kandel Writer Robert Yale Libott Writer Alf Kjellin Director Boris Ingster Writer