Hayley Atwell Agent Peggy Carter Actor James D'Arcy Edwin Jarvis Actor Enver Gjokaj Agent Daniel Sousa Actor Wynn Everett Whitney Frost Actor Reggie Austin Jason Wilkes Actor Chad Michael Murray Chief Jack Thompson Actor Currie Graham Guest Star Lotte Verbeek Guest Star Lesley Boone Guest Star Sarah Bolger Guest Star Bridget Regan Guest Star Sean O'Bryan Guest Star John Gilbert Guest Star Kurtwood Smith Guest Star Edward Deraney Guest Star Kevin Ashworth Guest Star Angela Cristantello Guest Star Bruce Katzman Guest Star Alex Alcheh Guest Star Matt Braunger Guest Star Jonathan LaVallee Guest Star Tara Butters Executive Producer Michele Fazekas Executive Producer Christopher Markus Executive Producer Stephen McFeely Executive Producer Chris Dingess Executive Producer Kevin Feige Executive Producer Louis D'Esposito Executive Producer Alan Fine Executive Producer Joe Quesada Executive Producer Stan Lee Executive Producer Jeph Loeb Executive Producer Brant Englestein Writer Lawrence Trilling Director