Hayley Atwell Agent Peggy Carter Actor James D'Arcy Edwin Jarvis Actor Chad Michael Murray Agent Jack Thompson Actor Enver Gjokaj Agent Daniel Sousa Actor Shea Whigham Chief Roger Dooley Actor Lyndsy Fonseca Guest Star Dominic Cooper Guest Star Andre Royo Guest Star James Landry Hébert Guest Star Kyle Bornheimer Guest Star Ashley Hinshaw Guest Star Carrick O'Quinn Guest Star James Frain Guest Star Tim True Guest Star Johnny Marques Guest Star Jeffrey David Anderson Guest Star James Urbaniak Guest Star Bill Kalmenson Guest Star Lesley Boone Guest Star Costa Ronin Guest Star Kevin Heffernan Guest Star Tara Butters Executive Producer Michele Fazekas Executive Producer Christopher Markus Executive Producer, Writer Stephen McFeely Executive Producer, Writer Chris Dingess Executive Producer Kevin Feige Executive Producer Louis D'Esposito Executive Producer, Director Alan Fine Executive Producer Joe Quesada Executive Producer Stan Lee Executive Producer Jeph Loeb Executive Producer