Robert Vaughn Napolean Solo Actor David McCallum Illya Kuryakin Actor Leo G. Carroll Mr. Alexander Waverly Actor Henry Jones Guest Star Jeremy Slate Guest Star Marta Kristen Guest Star Alexander Lockwood Guest Star John Banner Guest Star May Heatherly Guest Star John Harding Guest Star Norman Felton Executive Producer Sam Rolfe Producer Vincent McEveety Director Henry Sharp Writer John W. Bloch Writer